TY - JOUR A1 - Pack, Andreas A1 - Höweling, Andres A1 - Hezel, Dominik C. A1 - Stefanak, Maren T. A1 - Beck, Anne-Katrin A1 - Peters, Stefan T. M. A1 - Sengupta, Sukanya A1 - Herwartz, Daniel A1 - Folco, Luigi T1 - Tracing the oxygen isotope composition of the upper Earth's atmosphere using cosmic spherules Y1 - 2017-06-01 VL - 8 SP - 15702 EP - 15702 JF - Nature communications DO - 10.1038/ncomms15702 DO - 10.23689/fidgeo-2741 N2 - Molten I-type cosmic spherules formed by heating, oxidation and melting of extraterrestrial Fe,Ni metal alloys. The entire oxygen in these spherules sources from the atmosphere. Therefore, I-type cosmic spherules are suitable tracers for the isotopic composition of the upper atmosphere at altitudes between 80 and 115 km. Here we present data on I-type cosmic spherules collected in Antarctica. Their composition is compared with the composition of tropospheric O2. Our data suggest that the Earth's atmospheric O2 is isotopically homogenous up to the thermosphere. This makes fossil I-type micrometeorites ideal proxies for ancient atmospheric CO2 levels. UR - http://resolver.sub.uni-goettingen.de/purl?gldocs-11858/7054 ER -